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Comparative analysis of experimentally measured Raman spectra of crystalline (c), glassy (g), and powdered c‐As2S3 samples is performed based on vibrational modes of As6S6+6/2 ring‐like nanoclusters being fully (“rigid”) or partially (“soft”) interconnected with the glassy matrix, calculated using density functional theory (DFT). Although good agreement is found in the 100–500 cm−1 spectral range,...
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