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A molecular Mott insulator β′‐EtMe3Sb[Pd(dmit)2]2 with a quasi‐triangular lattice of a dimer unit [Pd(dmit)2] exhibits quantum spin liquid (QSL) behavior. We introduced Me4Sb+ or Et2Me2Sb+ to the cation site of this anion radical salt without altering its crystal symmetry. The mixing ratio and lattice parameters of these mixed crystals can be continuously tuned. We calculated intermolecular transfer...
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