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Adamantine ternary ordered‐vacancy compounds (OVCs) of the AB2X4 family derive from the zincblende structure of binary AX compounds and share many properties with the chalcopyrite‐type ternary ABX2 compounds. AB2X4 mainly crystallize in the defect chalcopyrite (or thiogallate) structure but also in other vacancy‐ordered phases, like the defect stannite (DS, or defect famatinite) and the pseudocubic...
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