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Cycloadditions of silylenes (silicon analogues of carbene) have been extensively explored as convenient and efficient routes to silacycles. Among these, reactions of silylenes with nitriles are still limited and the electronic properties of the resulting azasilacycles such as 2H‐azasilirene and 1,3‐diaza‐2‐siloles are less examined. We report herein synthesis of a phenylene‐bridged 1,3‐diaza‐2‐silole...
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