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Reactions of (dien)M 2+ (M=Pt, Pd) with cytosine (CH) lead to mixtures of linkage isomers with N3 and N1 bonded metal entities as well as N3,N1 bridged species, as demonstrated by 1 H NMR spectroscopy. The N3 linkage isomer is preferred over the N1 linkage isomer throughout the pH range studied (2.5–9), but the ratio does not parallel the equilibrium constant between the aminooxo tautomer...
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