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Interest in Criegee intermediates (CIs), often termed carbonyl oxides, and their role in tropospheric chemistry has grown massively since the demonstration of laboratory‐based routes to their formation and characterization in the gas phase. This article reviews current knowledge regarding the electronic spectroscopy of atmospherically relevant CIs like CH2OO, CH3CHOO, (CH3)2COO and larger CIs like...
The results of recent mass-resolved resonance enhanced multiphoton ionisation (REMPI) and REMPI-photoelectron spectroscopy (PES) studies of the sixteen valence electron molecules OCS and CS 2 are used to illustrate some of the many opportunities offered by (and a few of the possible limitations associated with) these techniques when applied to studies of the spectroscopy and the decay dynamics...
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