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Polycrystalline bilayer thin film of multiferroic [Ba(Zr0.2Ti0.8)O3‐0.5(Ba0.7Ca0.3)TiO3]/CoFe2O4([BZT‐0.5BCT]/CFO) has been deposited on Pt/Si (100) substrate using a pulsed laser deposition technique. The dielectric analysis reveals a significant change in the dielectric constant (~39% at a typical frequency of 100 Hz) at room temperature when a magnetic field is applied, in addition to a substantial...