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Herein, a simple and green quasi‐solid‐phase (QSP) method for facile synthesis of proton‐type ZSM‐5 avoiding use of excessive water, dry gel, Na+ cation and fluoride is reported. Crystallization by using the stoichiometric amount of TPAOH (tetrapropylammonium hydroxide) at 180 °C for only 12 h gave well‐structured HZSM‐5 crystals with high specific surface area of 429 m2 g−1 and high thermal stability...