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An influential method for the synthesis of imidazo[2,1‐b]thiazoles via copper (I) catalysis was advanced through a multicomponent coupling of pharmacological scaffolds involving 2‐aminothiazolyl‐coumarin, benzaldehyde, and phenyl acetylene, a concealed variation. The protocol allows the establishment of highly efficient and user‐friendly catalytic system for the A3 cascade coupling; also, an environmentally...