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Breaking the D4h symmetry in the square‐planar M−N4 configuration of macrocycle molecular catalysts has witnessed enhanced electrocatalytic activity, but at the expense of electrochemical stability. Herein, we hypothesize that the lability of the active Cu−N3 motifs in the N‐confused copper (II) tetraphenylporphyrin (CuNCP) could be overcome by applying pulsed potential electrolysis (PPE) during electrocatalytic...
Breaking the D4h symmetry in the square‐planar M−N4 configuration of macrocycle molecular catalysts has witnessed enhanced electrocatalytic activity, but at the expense of electrochemical stability. Herein, we hypothesize that the lability of the active Cu−N3 motifs in the N‐confused copper (II) tetraphenylporphyrin (CuNCP) could be overcome by applying pulsed potential electrolysis (PPE) during electrocatalytic...
Vapor-phase esterification of cellulose was achieved by exposing filter paper and tunicate cellulose film to mixed vapor of trifluoroacetic anhydride (TFAA) and acetic acid (AcOH) or TFAA and acetic anhydride (Ac2O) at room temperature. Both treatments gave high hydrophobicity to the specimens. The hydrophobicity of TFAA/AcOH-treated sample was resistant to water immersion, but that of TFAA/Ac2O-treated...
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