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Development of low‐cost electrocatalysts for water splitting is crucial to economical hydrogen production. Here, a highly efficient electrocatalyst composed of MoNi4‐embedded amorphous MoO2 nanosheets grown on less‐tortuosity hierarchically porous carbonized wood (MoNi4/MoO2@CW) is reported. The generation of abundant MoNi4/MoO2 heterointerfaces and defects‐rich MoO2 significantly promote the adsorption...