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We describe here the first report of a metallacarborane complex as a redox mediator in a functioning biofuel cell. Specifically, we have prepared a water-soluble salt of the complex anion [commo-3,3′-Fe-(closo-2,1-C 2 B 9 H 11 ) 2 ] − and employed it as a redox mediator for glucose oxidation using chitosan/multiwalled carbon nanotube-modified electrodes comprising...