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Polydopamine (PDA)/casein phosphopeptide (CPP) bilayers were prepared on titanium (Ti) substrates through a simple two-step immersion process at room temperature. The adhering PDA interlayers linked the natural biomolecule, CPP, to the Ti surface via covalent bonds. The outer layer of CPP served as a template to bind Ca2+ and thus promoted nucleation and growth of hydroxyapatite (HA). Our results...