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Large-area (approximately 1 cm 2 ) mosaic diamond substrates were obtained by orienting smaller (250 μm on a side) diamond cubes and fusing them homoepitaxially. The orientation starts by distributing a single layer of several hundred cubes on a smooth substrate. The cubes are then wetted with a mixture of isopropyl alcohol and glycerin, whose surface tension causes the cubes to coalesce into...