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Horseradish peroxidase (HRP) is well known for mediating the electron-transfer oxidation of electron-rich aromatic donors such as phenols and anilines, but has not been described to oxidize aliphatic amines. We here confirm the inability of HRP to oxidize typical aliphatic amines, even those which would exist significantly as free bases at the operative pH. In contrast, trans-2-phenylcyclopropylamine...