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CuH-catalyzed 1,2-additions to β,β-disubstituted α,β-unsaturated ketones have been further explored. Asymmetric reductions of enones lacking an α-substituent can be achieved with CuH complexed by DTBM-SEGPHOS in Et 2 O at −25°C leading to the generation of highly valuable nonracemic allylic alcohols. The corresponding 1,4-reductions can also be achieved using the same reaction conditions by...
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