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Memristors‐based integrated circuits for emerging bio‐inspired computing paradigms require an integrated approach utilizing both volatile and nonvolatile memristive devices. Here, an innovative architecture comprising of 1D CVD‐grown core–shell heterostructures (CSHSs) of MoO2‐MoS2 is employed as memristors manifesting both volatile switching (with high selectivity of 107 and steep slope of 0.6 mV decade...