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Recrystallization is usually required for the application of 2,6‐Diamino‐3,5‐dinitropyrazine‐1‐oxide (LLM‐105) as an energy material due to its poor crystal morphology. The study of its solubilities in binary solvent mixtures can provide primary support for optimizing the recrystallization and spheroidization conditions of LLM‐105. In the current work, the solubilities of LLM‐105 in the binary mixtures...