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In this work, composite samples were fabricated through melt blending with mesocarbon microbeads (MCMBs) and polyamide‐66 (PA66). Noteworthily, the thermal conductivity (TC) of the composites reached 1.51 W/m K with 60 wt% MCMBs, and the mechanical properties and heat resistance of PA66/MCMB composite were significantly improved. It was mainly due to the formation of heat transfer network at high...