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Two series of electron‐rich metal (Ni and Pd) complexes, namely a pyridine‐coordinated tridentate NHC/amidate/phenoxy metal complex and a tetradentate complex bearing an extra pyridyl group, were synthesized. Two carbene moieties, imidazole‐based and benzimidazole‐based NHCs, were also incorporated into the ligand backbones. Seven of the new complexes were structurally characterized and comparative...