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Telluronium salts [Ar2MeTe]X were synthesized, and their Lewis acidic properties towards a number of Lewis bases were addressed in solution by physical and theoretical means. Structural X‐ray diffraction analysis of 21 different salts revealed the electrophilicity of the Te centers in their interactions with anions. Telluroniums’ propensity to form Lewis pairs was investigated with OPPh3. Diffusion‐ordered...