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The ability to imprint a given material property to another through a proximity effect in layered 2D materials has opened the way to the creation of designer materials. Here, molecular‐beam epitaxy is used for direct synthesis of a superconductor–ferromagnet heterostructure by combining superconducting niobium diselenide (NbSe2) with the monolayer ferromagnetic chromium tribromide (CrBr3). Using different...