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Several phosphaquinodimethanes and their M(CO)5 complexes (M=Cr, Mo, W) and model derivatives have been theoretically investigated regarding the quest of non‐innocence. Computed structural and electronic properties of the P‐Me/NH2 substituted phosphaquinodimethanes and tungsten complexes revealed an interesting non‐innocent ligand behaviour for the radical anion complexes with distonic ion character...
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