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The photolysis of 3-cyclopentenone adsorbed on MgF 2 at 193 nm has been investigated. B state resonance-enhanced multi-photon ionisation spectroscopy was used to probe the vibrational and rotational state of the desorbed CO. The vibrational distribution of the CO is the same as that determined under collision-free conditions in the gas phase. The majority of the desorbed molecules show...