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Ytterbium tri-fluoromethanesulfonate (YbTFMS) single crystals are prepared from the slow evaporation of the aqueous solution of YbTFMS and the principal magnetic susceptibility perpendicular to the c-axis of the hexagonal crystal (χ ⊥ ) is measured from 300K down to 13K. Principal magnetic anisotropy Δχ(=χ ∥ −χ ⊥ ) is measured from 300K down to 80K which provides principal...