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In this contribution we present the structural and optical properties of small noble‐metal clusters at the FS‐center defect of the MgO (100) support. We focus on comparing absorption and emission properties of supported silver and gold clusters. It will be shown that the leading absorption features in the low energy regime are similar for supported silver and gold clusters of the same size, in spite...
We present a theoretical study of the ultrafast dynamics in noble metal clusters interacting with molecular oxygen which is of fundamental importance for the understanding and design of cluster-based heterogenous nanocatalysts. We demonstrate that intrinsic dynamical properties can significantly promote the reactivity of small noble metal clusters towards O 2 . This concept is illustrated...
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