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The dehydrocyclisation ofn-hexane to benzene has long been reported to be selectively catalysed by Pt-KL and other Pt impregnated basic zeolites. In this contribution, Pt-impregnated basic microporous titanosilicates ETS-10 and ETAS-10 are shown to catalyse this reaction with remarkably high selectivities. Although these two materials are topologically identical, their catalytic performance differs...