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The anisotropy barrier and blocking temperature of single-molecule magnets (SMMs) depend on the total spin S (and therefore to some extent on the size of the molecule) as well as on the Ising-type axial magnetic anisotropy D. There is a relatively large anisotropy of the magnetic exchange across cyanide bridges and therefore, moderate-sized oligonuclear complexes may lead to appreciably high anisotropy...
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