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Perturbation solution of the Boltzmann equation for a dilute gas with a chemical reaction A + A → B + B is presented. Analytical results for the nonequilibrium effects on the rate of chemical reaction are obtained for the line-of-centers model. It is shown that taking into account the energy transfer from reagents A to products B permits to get new results. The nonequilibrium corrections obtained...
A simple approach to the process of translational energy relaxation in dilute gases due to Dahler, Malkin, Shizgal and others is extended to the case of systems with chemical reaction. Fundamental quantities characterizing the relaxation processes such as the relaxation time and collision numbers during this time are computed for a number of molecular models of the chemical reaction (the Prigogine-Xhrouet...
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