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The sulfur, oxygen and chlorine atom transfer reactions of thio-W(VI) and -W(IV) complexes containing monodentate and ambidentate dithiophosphinate co-ligands are examined. Systems featuring monodentate ligands are complicated by the instability of the W(IV) species; significantly and in contrast to observations in thio-Mo chemistry, thio-W(VI) complexes such as Tp*WS 2 Cl fail to react with...
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