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In the first paper from this series we pointed out that the stereoselectivity in the reduction of benzaldehyde with B-alkyl-9-BBN reagents greatly depends on the borane reagent conformations. The AM1 calculations show that the stereoselectivity in the reduction of acetophenone with a series of B-Ipc-BYX reagents is also controlled by the borane conformations. It appears that this control is imposed...
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