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The performance of a silica sol–gel biosensor is intimately related to the characteristics of an encapsulated guest molecule. The effect of charge, size, and polarity on the behavior of the encapsulate was investigated using both ensemble measurements and single-molecule spectroscopy. Simply by monitoring the mobility of individual encapsulates, the heterogeneous microscopic environment within a silica...
Dye aggregation is detrimental to the performance of high optical density dye-doped photonic materials. To overcome this challenge, the ability of cucurbit[7]uril (CB7) as a molecular host to disrupt aggregate formation on glass substrates was examined. Rhodamine B was covalently attached to glass slides by initially coating the surface with azidohexylsiloxane followed by copper-catalyzed “click”...
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