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Solid‐contact ion‐selective electrodes with thin membranes can more easily achieve complete ion exchange at the sample‐membrane interface, giving unbiased selectivity coefficients. The calculated reconditioning rate corresponds well to experimental data. Alternatively, the redox state of the conducting polymer may be electrochemically switched resulting in primary ion expulsion from the membrane and...
A generalized description of the response behavior of potentiometric polymer membrane ion-selective electrodes is presented on the basis of ion-exchange equilibrium considerations at the sample–membrane interface. This paper includes and extends on previously reported theoretical advances in a more compact yet more comprehensive form. Specifically, the phase boundary potential model is used to derive...
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