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Electrocatalysts facilitating chlorine evolution reaction (ClER) play a vital role in chlor–alkali industries. Owing to a huge amount of chlorine consumed worldwide, inexpensive high‐performing catalysts for Cl2 production are highly demanded. Here, a superb ClER catalyst fabricated through uniform dispersion of Pt single atoms (SAs) in C2N2 moieties of N‐doped graphene (denoted as Pt‐1) is presented,...