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Three phosphonium polyelectrolytes have been prepared wherein the flexibility of the spacer between charge‐bearing phosphonium units was varied from 1,2‐ethyl to 1,4‐phenyl to 1,1′‐ferrocenyl. The influence of inter‐phosphonium spacer flexibility on the ability of the polyelectrolyte to form ordered films via layer‐by‐layer supramolecular assembly with anionic polythiophene and anionic poly(p‐phenylenevinylene)...
Two π‐conjugated polymers featuring main‐chain m‐phenylene linkers as well as iodo substituents were initially prepared. The presence of the iodo functionality allowed for the preparation of six additional polymers from the initial two iodo‐substituted polymers via facile post‐polymerization modification using Sonogashira‐type coupling chemistry. The post‐polymerization modification led to crosslinking,...
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