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A series of novel 2D‐D‐π‐A‐type organic dyes, namely CCTTnA (n = 1–3), bearing bis(3,6‐di‐tert‐butylcarbazol‐9‐ylphenyl)aniline as an electron‐donor moiety (2D‐D), oligothiophene segments with a number of thiophene units from one to three units as π‐conjugated spacers (π), and cyanoacrylic acid as the electron acceptor (A) were synthesized and characterized as dye sensitizers for dye‐sensitized solar...