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In this study, in situ modified cyclohexanone formaldehyde resin (CFR) was prepared from clay (montmorillonite) and polydimethylsiloxane with diamine chain ends [α,ω‐diamine poly(dimethyl siloxane) (DA.PDMS)] in the presence of a base catalyst. Different clay contents (from 0.5 to 3 wt %) were used to produce clay‐modified nanocomposite ketonic resins [layered clay (LC)–CFR] and clay‐ and DA.PDMS‐modified...