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MXenes have recently been used to grow highly textured potassium niobate ferroelectric crystals. Herein, the versatility of MXenes is further demonstrated by growing ferroelectric and luminescent lithium niobate (LiNbO3) crystals from niobium carbide MXene (Nb2CTx). The formation of high‐aspect‐ratio LiNbO3 rhombic crystals is confirmed by extensive structural analysis. The ferroelectricity of MXene‐derived...