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In this paper, in order to develop the composition ceramics for piezoelectric actuator. (1 − x)(Na0.52K0.443Li0.037)(Nb0.883Sb0.08Ta0.037)O3 − x(Sr0.95Ca0.05)ZrO3 ceramics were sintered at 1020 °C by the conventional solid-state method. The effects of (Sr0.95Ca0.05)ZrO3 substitution on their microstructure and piezoelectric properties were systematically investigated. The orthorhombic-tetragonal coexistence...