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A novel cellulose and chitosan-based natural biopolymer or coagulant aids with a commercial coagulant (ferric chloride FeCl3) have been used for the removal of arsenite As(III) from synthetic tap water at 2 mg/L of initial arsenic concentration by coagulation–flocculation method. The maximum As(III) removal efficiency of 69.25% was obtained without coagulant aids at 40 mg/L concentration of FeCl3...