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Galactose oxidase is a type II copper protein that contains a square–pyramidal five-coordinate copper center and catalyzes the oxidation of primary alcohols to aldehydes with a concomitant reduction of molecular oxygen. Dimeric (4-methylpyridine-N)(N-salicylidene-tyrosinato-O, N, O′)copper(II), which contains two square–pyramidal five-coordinate copper centers and thus serves as a model for galactose...