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A novel strategy for the synthesis of 6‐methyl benzofuro[3,2‐c] quinoline derivatives via copper‐catalyzed dehydrogenative CO arylation has been presented. Optimization studies have been carried out by varying various catalysts, bases, solvents, and other physical parameters. Keeping use of this dehydrogenative cross‐coupling CO arylation reaction, a variety of bioactive building blocks like fused...