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A thorough statistical mechanical analysis of sources of variations and correlations in ΔE0 and ΔS0 of spin crossover equilibrium in the solid state is given. Attention has been brought to possible contributions of vibrations and rotations towards the entropy of reaction. In the ideal approximation, isoequilibrium relationships (IER) can be observed due to variations in the intermediate-frequency...
A thorough statistical mechanical analysis of sources of variations and correlations in ΔE0 and ΔS0 of spin crossover equilibrium in the solid state is given. Attention has been brought to possible contributions of vibrations and rotations towards the entropy of reaction. In the ideal approximation, isoequilibrium relationships (IER) can be observed due to variations in the intermediate-frequency...
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