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Polycrystalline thin films of highly Bi substituted Dy iron garnets, [(BixDy3−x(Fe, Ga)5O12], with [111] crystalline orientation perpendicular to the film plane were grown on (111) Gd3Ga5O12, single crystal substrates using pulsed laser deposition technique. In the deposited films, Bi stoichiometry was found to be very sensitive to both substrate temperature and oxygen pressure. The Bi volatilisation...