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We have reviewed the experimental and theoretical studies of mechanisms by which the energy gap dependence of the electron transfer rate differs between the photoinduced charge separation and the charge recombination reactions in solution. Also how much the distance distribution between donor and acceptor, the quantum effect of the intramolecular vibration and the non-linear response effect of solvent...
Viability of the analysis using the Collins-Kimball model for the rate constant of photoinduced charge separation reactions in polar solutions is investigated. In the Collins-Kimball model, it is assumed that the reaction occurs only at a specified distance in the encounter between donor and acceptor molecules under mutual diffusional motion while in real systems the reaction can occur over a range...
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