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The adsorption of binary mixtures on heterogeneous surfaces is studied by a cluster approximation (CA), based on the exact calculation of configurations on finite cells. The substrate is characterized by n types of sites, each with different adsorption energy. The process is monitored through the total and partial isotherms. The theoretical formalism is used to model experimental data of methane–ethane...
Adsorption and collective diffusion of interacting particles on one-dimensional heterogeneous lattices are studied by both Monte Carlo simulation and theoretical modeling (cluster approximation). The heterogeneous substrate is modeled as a chain of adsorptive sites with patchwise topography. Patches of equal size are alternatively distributed with adsorption energies E 1 and E 2 (bivariate...
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