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In the past few years, many studies have reported on the formula of solder metal alloy materials. This paper discusses the influence of organic materials characters, the decomposing rate of flux in lead-free solder paste and coefficients of thermal expansion (CTE) of halogen-free mold compounds during the on-board reliability test, and the failure mechanism in both 63Sn/37Pb and Sn–3.5Ag–0.5Cu lead-free...