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In the family of pseudo binaries, xAlCl 3 -(1-x)MSCN (M = Li, Na, or K), ambient-temperature molten salt solutions are formed over the composition range, 0.35 < x < 0.75. These molten salt solutions readily form glasses. A partial determination of the phase equilibria for these pseudo binaries was made. For all three A1C1 3 -MSCN systems, a eutectic occurs at ~65 mol % AICl ...