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Photoelectron-photoion coincidence (PEPICO) spectra at 73.6 nm reveal an interesting fact; from hexafluorobenzene cation the C 5 F 3+ fragment is most abundant whilst from the benzene cation C 4 H 4+ is far more abundant than C 5 H 3+ . These contrasting results are connected, as shown by the PEPICO spectra of other fluorinated benzenes,...
Breakdown of the ions created by photoionisation of C 6 F 6 at 73.6, 58.4 and 30.4 nm has been examined by two separate photoelectron-photoion coincidence techniques and has been interpreted using density functional theory calculations. A full breakdown diagram, amplifying earlier metastable ion studies, is determined. The rate of the main dissociative rearrangement reaction forming...
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