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Liquid-state infrared (IR) and Raman spectra and solid-state IR spectra were obtained for 2-methyl-1-pentene. Vibrational assignments were made for all four possible conformers with the aid of normal coordinate calculations. The trans-trans (TT) and trans-gauche (TG) conformers were both found to be present in the unannealed solid, but only the TT conformer was present in the annealed (crystalline)...